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Has anyone tried learning/taking the enchantments off of the thieves and dark brotherhood armor so they could enchant some better gear with the same effects?
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They cannot. Many unique items cannot be disenchanted. Weirdly Linwe's armor can be, teaching you unique enchantments like Shadowstrike and Shadowsight, though this appears to be an oversight on the part of the developers because they can't actually be applied to any item.
However you can recreate them. Most, if not all of these effects exist as other enchantments on ordinary items. I'm currently raising my enchantment and alchemy skills so that I can put two powerful enchantments on every item of apparel. Not sure which ones yet, though I'm thinking of stacking four instances of Fortify Health Regeneration and Fortify Stamina Regeneration.
Incidentally, there are four item types that can be enchanted with the Fortify [School of Magic] effect which reduces the Magicka cost of those kinds of spells. And the best effect possible is 25% reduction. Free spells, anyone? Elemental Destruction perks and Fortify enchantments also affect the appropriate elemental weapon enchantments. Which means the Fire Damage perks in Destruction improve created Fire Damage enchantments on weapons, and all four 25% Fortify Destruction enchantments on clothes will make enchanted weapons consume no charge when used.
I've been experimenting.