Alexander DeLarge was a good character, but I wouldn't call him a villain in the true sense. When I think of Villains, I tend to think of; Darth Vadar, Agent Smith, The Terminator (the evil ones), Cohagen from the Total Recall film, the orcs in LOTR...
I think Bowser is the daddy when it comes to videogame villains. He's kidnapped the princess at least thirteen times in 20+ years!!!
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