PS1:
Heart Of Darkness.
Ghost In The Shell.
Tombi (Very rare, would be expensive if you could find it).
Dragon Valor (A little Hack 'n' Slash but still very good).
Jade Cocoon (The original mind you, 2 was a disappointment).
Ape Escape.
Silent Hill (Only if you like horror/puzzle games).
Resident Evil 2 (Same reason as Silent Hill).
Star Ocean the second story.
Medieval.
PS2:
Time Splitters 2.
Guitar Hero Series (3rd is the best).
You must try Dark Cloud or Dark Chronicle before you buy them, I found the games to be extremely repetitive, I gave up on Dark Cloud when I discovered the second area of the game was almost exactly the same as the first, only harder.
Strangely enough I can't think of many PS2 games. I'll add more if I can think of any.
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