Oooh... tough. Very tough.
I'm tempted to say Silent Hill 2, because it was probably the most atmospheric game I've ever played. It created a world unto it's own, a virtual nightmare.
Strictly going by time spent playing, I would have to say The Elder Scrolls 3: Morrowind. That sucked my life up in high school.
Shadow of the Colossus, Fatal Frame 2, and Battlefield 2 all deserve mention, but I'll have to go with Silent Hill 2.
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